Charisma & Friends Spell
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I also know that a High Charisma impacts discounts (as has already been mentioned) and will impact NPC reactions (like Viconia deciding to join etc...).
Like you, I would have preferred these factors to do more. I envisioned that casting Friends spells on AGRO'd pick pocket victims would smooth things over. And I even imagined that the spell would effect Merl in Bergost, but I don't think it does. More's the pity.
But yes, charisma is polled a lot of places in dialogues, though not necessarily directly. Many NPCs will have different dialogue paths and quest rewards based upon their reaction to you, of which one component is charisma (the other is reputation). There's also the aforementioned store discounts for high charisma as well.